Research Topics
| John M SimmieSummaryAffiliation: National University of Ireland Country: Ireland Publications
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Detail Information
Publications
Enthalpies of formation and bond dissociation energies of lower alkyl hydroperoxides and related hydroperoxy and alkoxy radicalsJohn M Simmie
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
J Phys Chem A 112:5010-6. 2008..We recommend a new set of group additivity contributions for the estimation of enthalpies of formation and bond energies...
Formation enthalpies and bond dissociation energies of alkylfurans. The strongest CX bonds known?John M Simmie
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
J Phys Chem A 113:5128-37. 2009..These results have implications for the construction of detailed chemical kinetic models to account for the thermal decomposition and oxidation of alkylfurans either in engines or in the atmosphere...
Harmonising production, properties and environmental consequences of liquid transport fuels from biomass--2,5-dimethylfuran as a case studyJohn M Simmie
Combustion Chemistry Centre, School of Chemistry, National University of Ireland, Galway, Ireland
ChemSusChem 6:36-41. 2013..A primary consideration is to avoid a repetition of the methyl tert-butyl ether (MTBE) fiasco...
Kinetics and thermochemistry of 2,5-dimethyltetrahydrofuran and related oxolanes: next next-generation biofuelsJohn M Simmie
Combustion Chemistry Centre, School of Chemistry, National University of Ireland, Galway, Ireland 091
J Phys Chem A 116:4528-38. 2012..It is probable that the compounds at the center of this study will be relatively clean-burning biofuels, although formation of intermediate aldehydes might be problematic...
Energy barriers for the addition of H, *CH3, and *C2H5 to *CH2=CHX [X = H, CH3, OH] and for H-atom addition to RCH=O [R = H, CH3, *C2H5, n-C3H7]: implications for the gas-phase chemistry of enolsJohn M Simmie
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
J Phys Chem A 113:7834-45. 2009..8 +/- 1.6, -151.8 +/- 1.7, and -169.9 +/- 1.5 kJ mol(-1), respectively, are proposed...
Ab initio study of the decomposition of 2,5-dimethylfuranJohn M Simmie
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
J Phys Chem A 115:8877-88. 2011..Identification of 2-ethenylfuran as an C(6)H(6)O intermediate in 2,5-dimethylfuran flames is probably not correct and is more likely the isomeric 2,5-dimethylene-2,5-dihydrofuran for which credible formation channels exist...
Ab initio chemical kinetics of methyl formate decomposition: the simplest model biodieselWayne K Metcalfe
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
J Phys Chem A 114:5478-84. 2010..15 K) of -360.1 +/- 2.2 kJ mol(-1). In turn, bond dissociation energies for all single bonds in the molecule are presented...
Ab initio and kinetic study of the reaction of ketones with OH for T = 500-2000 K. Part I: hydrogen-abstraction from H3CC(O)CH(3-x)(CH3)x, x = 0 ↦ 2Chong Wen Zhou
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
Phys Chem Chem Phys 13:11175-92. 2011..32 × 10(2)×T(3.30)exp(503/T), k(EMK) = 3.84 × 10(1)×T(3.51)exp(1515/T), k(iPMK) = 2.08 × 10(1)×T(3.58)exp(2161/T). Group rate constants (on a per H atom basis) for different carbon sites in title reactions have also been provided...
Enthalpies of formation, bond dissociation energies and reaction paths for the decomposition of model biofuels: ethyl propanoate and methyl butanoateAhmed M El Nahas
Chemistry Department, National University of Ireland, Galway, Ireland
J Phys Chem A 111:3727-39. 2007..Propene formation is a much higher energy demanding process, 402 kJ mol(-1), and it should be competitive with some C-C, C-O, and C-H bond cleavage processes...
Barrier heights for H-atom abstraction by H*O2 from n-butanol--a simple yet exacting test for model chemistries?Gráinne Black
Combustion Chemistry Centre, National University of Ireland, Galway, Ireland
J Comput Chem 31:1236-48. 2010..However, the absolute values obtained do not agree that well with the benchmarks; the composite G3 method predicts the correct order and comes closest (< or = 2 kJ, mol (-1)) in absolute numerical terms for H-abstraction from carbon...
